If you don't have the patience to slowly fill the void with spray foam through holes drilled in one of the studs, you could (if you were an experienced carpenter) use a Sawzall to remove one of the studs and re-frame the corner as a two-stud corner. Then you could either insulate the void with a fiberglass batt or simply present the two-stud corner to the spray-foam contractor as an accessible corner. http://youtube.com/watch?v=ggLAUsiuI_o&app=desktop

Closed-cell (aka two-pound foam) is denser than open-cell at about 2 pounds per cubic foot. Its R-Value is between 6-6.5 per inch. As a result, this kind of foam is much more expensive than its counterpart. The reason closed-cell doesn't need a vapor retarder is because it already has one. It's permeance is 0.8 perm, which means it can handle cold climates without the use of an additional board or drywall. Closed-cell uses hydroflurocarbons (HFCs) as part of its makeup. However, this material has been known to have a high global warming effect. If you want a green insulation solution, this is not the material to use. A way to avoid this and still use closed-cell is by installing it alongside fiberglass batts. https://youtube.com/watch?feature=player_embedded&v=ggLAUsiuI_o
Seal It Insulation Systems (headquartered out of Brunswick, Maine) performs residential home insulation, commercial spray foam insulation projects, and will also handle your industrial building needs. We use only the highest performing, industry tested foam products, with a primary focus on indoor air quality and temperature. While every insulation project is likely to give you a considerable return on your financial investment through gained energy efficiencies, it’s also likely to have a dramatic impact on your level of comfort. We work with homeowners, architects, contractors and facility managers to design these high-performing insulation systems, and to solve pre-existing performance issues in your building like ice damming, freezing pipes, high heating bills, mold/mildew conditions, and drafty, uncomfortable living spaces.
Loctite TITE FOAM Window and Door is a Loctite TITE FOAM Window and Door is a new generation of polyurethane-based insulating foam sealant that expands to fill seal and insulate around window and door jambs. Loctite TITE FOAM is a minimal-expanding foam based on purified and concentrated ingredients that provides four times more density versus conventional window and ...  More + Product Details Close

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once the foam is installed correctly, it is a inert plastic not much different than the foam cushions you sit on. there is not a health rick unless you have off ratio uncured foam that has not mixed properly. the foam is absolutely a health risk in its raw forms before it is mixed and cured. You should not be in the building without proper respirators and eye protection. The spray foam industry should be controlled and regulated by the same standards, testing and inspections that framing ,electrical and plumbing are. until that happens then you will have idiots with spray rigs ruining peoples homes and ruining the market for honest foam contractors that know how to price a job fairly and complete it correctly.
Spray foam insulation or spray polyurethane foam (SPF) is an alternative to traditional building insulation such as fiberglass. A two-component mixture composed of isocyanate and polyol resin comes together at the tip of a gun, and forms an expanding foam that is sprayed onto roof tiles, concrete slabs, into wall cavities, or through holes drilled in into a cavity of a finished wall.

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OK, Peter, I finally went back and read Alex Wilson's article on what he perceives as a serious problem. I haven't seen the full report, but based on the summary he wrote on the Green Building Advisor website, I question the science. It seems to me that he's chosen the wrong metric and he's basing his conclusion on too many assumptions because he doesn't have enough data. You can see my comments at the end of his article.

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This is in great contrast to my friend's experience. Her attic spaces were sprayed and the foam is actually pretty, and I was in her attic 6-7 days after it was sprayed and could hardly smell anything when I stuck my face up to the foam. And she did not have to clean up one speck of dust during or after the spraying. I got the name/number of the guy from her who managed her attic project, but between the time he did my house and the time he did her house, he was let go from the company who did her attic and hired by another company. He assured me everything would be the same, etc., etc., and I had no reason to believe anything had changed, but the sprayers who did my house later admitted they had never sprayed an attic before and I also found out that the foam used in my attic was from a different manufacturer. Neither my friend nor I had any idea this guy was with different company then, until the week after they filled my attic with off ratio foam, and my home with toxic vapors.  
Roof coatings are easy to install. Smaller roofs in good, serviceable condition can be a weekend do-it-yourself (DIY) project. Larger roofs with leaks and ponding water issues should be coated by a qualified professional. Additional roof coating products, such as foam or coatings designed for seams, may be required underneath the main coating layers. Supplement coating products are used to reinforce damaged or leak-prone problem areas.[3]
In a single application, Heatlok Soy 200 Plus can create a specialized engineered building envelope, which provides better thermal resistance, excellent air barrier, and a recognized vapor retarder. Demilec continues to strive toward innovative, scientific advancements in high-efficiency spray foam insulation solutions, intumescent and elastomeric coatings, high-performance quality products, and superior service.
SPF insulation applied by professionals is usually described as either a high- or low-pressure foam and is available as either open- or closed-cell. Each type has advantages and disadvantages depending on the application requirements. The comparison chart below can be helpful in explaining or understanding which type of SPF insulation is best suited to a specific application.
To avoid the expense re-roofing a house that is simply suffering from nail fatigue, and to obtain optimum insulation, an 85mm layer of polyurethane foam can be sprayed onto the underside of the slates or tiles of a pitched roof. This stabilises and weatherproofs the roof by fixing the nails, battens and roofing felt. As the foam is a superior insulant, coupled with just 100mm of insulation at joist level, your roof will also meet the stringent thermal performance standards required for a new home. A typical roof can be insulated using the polyurethane treatment for around half the cost of re-roofing.

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